- Bryce Papenbrook
- Â Meliodas / ... 74 episodes, 2014-2021
- Erika Harlacher
- Â Elizabeth / ... 73 episodes, 2014-2021
- Max Mittelman
- Â King 71 episodes, 2014-2021
- Cristina Valenzuela
- Â Hawk 67 episodes, 2014-2021
- Erica Mendez
- Â Diane 65 episodes, 2014-2021
- Ben Diskin
- Â Ban 60 episodes, 2014-2021
- Erik Scott Kimerer
- Â Gowther 56 episodes, 2015-2021
- Yûki Kaji
- Â Meliodas / ... 53 episodes, 2014-2021
- Rintarô Nishi
- Â Narration / ... 52 episodes, 2014-2018
- Misaki Kuno
- Â Hawk 51 episodes, 2014-2018
- Sora Amamiya
- Â Elizabeth / ... 48 episodes, 2014-2021
- Tatsuhisa Suzuki
- Â Ban 46 episodes, 2014-2021
- Robbie Daymond
- Â Glithunder / ... 46 episodes, 2014-2021
- Kaiji Tang
- Â Hendrickson / ... 46 episodes, 2014-2021
- Jun Fukuyama
- Â King 45 episodes, 2014-2021
- Aoi Yûki
- Â Diane 43 episodes, 2014-2021
- Kyle Hebert
- Â Escanor 42 episodes, 2018-2021
- Brianna Knickerbocker
- Â Elaine 37 episodes, 2014-2021
- Mamoru Miyano
- Â Gilthunder 33 episodes, 2014-2018
- Ryohei Kimura
- Â Howzer / ... 33 episodes, 2014-2018
- Abby Trott
- Â Veronica Liones / ... 33 episodes, 2014-2021
- Laura Megan Stahl
- Â Gerheade / ... 33 episodes, 2016-2021
- Chris Cason
- Â Fraudrin / ... 33 episodes, 2016-2020
- Allegra Clark
- Â Derieri / ... 33 episodes, 2018-2020
- Marina Inoue
- Â Jericho 32 episodes, 2014-2018
- Mela Lee
- Â Melascula 32 episodes, 2018-2020
- Yûya Uchida
- Â Hendrickson 31 episodes, 2014-2018
- Kayli Mills
- Â Deldry 30 episodes, 2018-2021
- Keith Silverstein
- Â Monspeet 30 episodes, 2018-2020
- Marin M. Miller
- Â Gloxinia 30 episodes, 2018-2020
- Billy Kametz
- Â Arden 29 episodes, 2018-2021
- Yûhei Takagi
- Â Gowther 28 episodes, 2014-2021
- Katsuyuki Konishi
- Â Dreyfus / ... 27 episodes, 2014-2018
- Lauren Landa
- Â Merlin / ... 27 episodes, 2014-2021
- Ray Chase
- Â Howzer / ... 26 episodes, 2014-2021
- Ray Carsillo
- Â Additional Voices 24 episodes, 2014-2015
- Robbie Friedman
- Â Additional Voices 24 episodes, 2014-2015
- Morgan Berry
- Â Daymond 24 episodes, 2018
- Maaya Sakamoto
- Â Merlin 23 episodes, 2015-2021
- Mariya Ise
- Â Guila / ... 21 episodes, 2014-2021
- Erica Lindbeck
- Â Jericho 20 episodes, 2014-2021
- Shin'ichirô Miki
- Â Slader 19 episodes, 2015-2018
- Genki Yoshimoto
- Â Holy Knight B / ... 19 episodes, 2014-2015
- Sachi Kokuryu
- Â Arthur 18 episodes, 2015-2018
- Ryûnosuke Watanuki
- Â Waillo / ... 18 episodes, 2018
- Jamieson Price
- Â Dreyfus / ... 18 episodes, 2014-2021
- Ben Lepley
- Â Deathpierce / ... 17 episodes, 2018-2021
- Hiroki Yamada
- Â Holy Knight A / ... 16 episodes, 2014-2015
- Carrie Keranen
- Â Guila / ... 16 episodes, 2014-2021
- Dorothy Elias-Fahn
- Â Margaret 16 episodes, 2015-2021
- Takahiro Sakurai
- Â Griamore 14 episodes, 2014-2018
- Zach Aguilar
- Â Arthur Pendragon / ... 14 episodes, 2015-2021
- Ken'ichirô Matsuda
- Â Taizoo / ... 13 episodes, 2014-2018
- Chris Hackney
- Â Gustav / ... 13 episodes, 2015-2021
- Kotori Koiwai
- Â Elaine 12 episodes, 2014-2018
- Ryôtarô Okiayu
- Â Helbram / ... 12 episodes, 2014-2015
- Yûsuke Kobayashi
- Â Gloxinia 12 episodes, 2018
- Hisako Kanemoto
- Â Veronica / ... 11 episodes, 2014-2018
- Kayô Nakajima
- Â Hawk Mama / ... 11 episodes, 2014-2018
- Patrick Seitz
- Â Griamore 11 episodes, 2016-2021
- Kirk Thornton
- Â Galand / ... 11 episodes, 2019-2021
- Nana Mizuki
- Â Margaret / ... 10 episodes, 2015-2018
- Hiroshi Iwasaki
- Â Galand 10 episodes, 2018
- Mao Ichimichi
- Â Melascula 10 episodes, 2018
- Emiri Kato
- Â Deldry / ... 10 episodes, 2014-2018
- Lucien Dodge
- Â Simon / ... 10 episodes, 2015-2021
- Griffin Burns
- Â Sariel 10 episodes, 2019-2020
- Bill Millsap
- Â Tarmiel 10 episodes, 2019-2020
- Tomokazu Sugita
- Â Escanor 9 episodes, 2018
- Shogo Yano
- Â Puora / ... 9 episodes, 2018
- Yui Nakajima
- Â Zeal / ... 9 episodes, 2015-2018
- Kenjirô Tsuda
- Â Monspiet 9 episodes, 2018
- Richard Epcar
- Â Helbram 9 episodes, 2014-2015
- Michael McConnohie
- Â Bartra / ... 9 episodes, 2016-2021
- David Vincent
- Â Estarossa / ... 9 episodes, 2019-2021
- Jordan Reynolds
- Â Ludociel 9 episodes, 2019-2020
- John DeMita
- Â Chandler 9 episodes, 2020-2021
- Rina Satô
- Â Matrona 8 episodes, 2018
- Himika Akaneya
- Â Jenna / ... 8 episodes, 2018
- Ayahi Takagaki
- Â Derieri 8 episodes, 2018
- Makoto Furukawa
- Â Gustaf 8 episodes, 2015-2018
- Minako Kotobuki
- Â Vivian 8 episodes, 2015-2018
- Marieve Herington
- Â Vivian / ... 8 episodes, 2015-2020
- Kyle McCarley
- Â Helbram / ... 8 episodes, 2015-2019
- Stephanie Sheh
- Â Zeal 8 episodes, 2015-2018
- Hiroshi Kamiya
- Â Helbram (Fairy) / ... 7 episodes, 2015-2018
- Ryôta Suzuki
- Â Knight / ... 7 episodes, 2018
- Takashi Inagaki
- Â Cain 7 episodes, 2014-2018
- Haruka Chisuga
- Â Zaneri / ... 6 episodes, 2018
- Toshiyuki Toyonaga
- Â Arden 6 episodes, 2018
- Yôhei Azakami
- Â Deathpierce 6 episodes, 2018
- Ryosuke Kanemoto
- Â Simon 6 episodes, 2015-2018
- Jason Marnocha
- Â Demon King 6 episodes, 2018-2021
- Mark Whitten
- Â Drole 6 episodes, 2019-2020
- Armen Taylor
- Â Cusack 6 episodes, 2020
- Chô
- Â Golgius 5 episodes, 2014-2018
- Yûko Hara
- Â Griamor (young) 5 episodes, 2015-2018
- Sumire Morohoshi
- Â Gerheade 5 episodes, 2018
- Hiroki Tôchi
- Â Estarossa 5 episodes, 2018
- Daisuke Ono
- Â Drole 5 episodes, 2018
- Hiromichi Tezuka
- Â Dogedo / ... 5 episodes, 2016-2018
- Doug Erholtz
- Â Slader 5 episodes, 2016-2021
- Megumi Han
- Â Freesia 4 episodes, 2014-2018
- Atsushi Ono
- Â Ruin 4 episodes, 2014-2018
- Jun'ichi Suwabe
- Â Zhivago 4 episodes, 2018
- Kôji Yusa
- Â Grayroad 4 episodes, 2018
- Tara Sands
- Â Young Ban / ... 4 episodes, 2014-2018
- Melissa Fahn
- Â Friesia 4 episodes, 2014-2018
- Landon McDonald
- Â Bartender 4 episodes, 2016
- Julia McIlvaine
- Â Nerobasta 4 episodes, 2018-2019
- Crispin Freeman
- Â Rou 4 episodes, 2019
- Greg Chun
- Â Gowther (Demon) 4 episodes, 2019
- Rikiya Koyama
- Â Zaratras 3 episodes, 2018
- Nobuyuki Hiyama
- Â Jude 3 episodes, 2014
- Mitsuru Miyamoto
- Â Dale / ... 3 episodes, 2014-2015
- Hidenobu Kiuchi
- Â Fraudrin 3 episodes, 2018
- Kazutomi Yamamoto
- Â Gilthunder (young) 3 episodes, 2014-2015
- Tomoyuki Shimura
- Â Dana 3 episodes, 2014
- Toshiki Iwasawa
- Â Customer B / ... 3 episodes, 2014
- Keisuke Kômoto
- Â Holy Knight B / ... 3 episodes, 2014-2015
- Ryôko Shiraishi
- Â Goddess / ... 3 episodes, 2015-2016
- Marc Diraison
- Â Ruin 3 episodes, 2014
- Jalen K. Cassell
- Â Jude 3 episodes, 2014
- Nozomi Furuki
- Â Ellen 3 episodes, 2014
- Lizzie Freeman
- Â Orlondi 3 episodes, 2019-2021
- Kenta Miyake
- Â Twigo 2 episodes, 2014
- Hideki Nakanishi
- Â Weinheidt 2 episodes, 2015
- Erika Sawai
- Â Jillian 2 episodes, 2015
- Daiki Hamano
- Â Nanashi 2 episodes, 2018
- Itaru Yamamoto
- Â Dumbelbas / ... 2 episodes, 2014-2018
- Masuo Amada
- Â Raizer 2 episodes, 2016-2018
- Shinobu Matsumoto
- Â Holy Knight B / ... 2 episodes, 2014-2015
- Austin Lee Matthews
- Â Additional Voices / ... 2 episodes, 2014
- Dave Mallow
- Â Golgius 2 episodes, 2014
- Taishi Murata
- Â Kairu Knights Leader 2 episodes, 2014
- Aiko Kusumi
- Â Child with Shakujo 2 episodes, 2014
- Bennett Abara
- Â The Trumpet of Carnanos / ... 2 episodes, 2015
- Shintarô Tanaka
- Â Pelio's Father / ... 2 episodes, 2016
- Kellen Goff
- Â Calmadios 2 episodes, 2019
- Xanthe Huynh
- Â Nadja 2 episodes, 2019
- Sayaka Ôhara
- Â Priestess of Chaos 2 episodes, 2021
- Hirofumi Nojima
- Â Alioni 1 episode, 2014
- Mamiko Noto
- Â Nerobasta 1 episode, 2018
- Mutsumi Sasaki
- Â Old Knight 1 episode, 2014
- Tetsuo Gotô
- Â Member A 1 episode, 2014
- Renpei Yasuda
- Â Group Member C 1 episode, 2014
- Ryô Hirohashi
- Â Dolores 1 episode, 2018
- Kenji Nojima
- Â Gannon 1 episode, 2018
- Kazuhiro Ãguro
- Â Giant 1 episode, 2018
- Shôzô Îzuka
- Â Demon King 1 episode, 2018
- Yumiko Kobayashi
- Â Mead 1 episode, 2014
- Takuya Masumoto
- Â Man C 1 episode, 2014
- Tôru Sakurai
- Â Knight B 1 episode, 2014
- Hikaru Ueda
- Â Boy 1 episode, 2014
- Minoru Yada
- Â Village Chief 1 episode, 2014
- Takuma Nagatsuka
- Â Girl 1 episode, 2014
- Yurie Kobori
- Â Cenette 1 episode, 2014
- Yasuyuki Sano
- Â Villager A 1 episode, 2014
- Yûichi Karasuma
- Â Villager E 1 episode, 2014
- Shin'ya Takahashi
- Â Holy Knight D 1 episode, 2015
- Makoto Takahashi
- Â Holy Knight C 1 episode, 2015
- Motoki Sakuma
- Â Holy Knight C 1 episode, 2015
- Sanae Fuku
- Â Fairy B 1 episode, 2015
- Sayuri Yahagi
- Â Pelio 1 episode, 2016
- Ikuji Nose
- Â Townsperson B 1 episode, 2016
- Kaho Kôda
- Â Pelio's Mother 1 episode, 2016
- Jonathan Fahn
- Â Golgius 1 episode, 2018
- Steve Kramer
- Â Cain 1 episode, 2019
- Brandon Jay
- Â Young Bartia 1 episode, 2019
- Katabelle
- Â Children's Voices / ... 1 episode, 2019
- David Errigo Jr.
- Â Young Estarossa 1 episode, 2020
- Amber Lee Connors
- Â Gelda 1 episode, 2021
- Mike McFarland
- Â Wild 1 episode, 2021
- Mikako Komatsu
- Â Tristan 1 episode, 2021
- Patrick Bach
- Â Meliodas (german version) (2015) unknown episodes